We are very pleased to welcome Bennet Karetta to the INSPIRE group. He joins the group as a M.Sc. Candidate joint with the TWIST group. We are looking forward to a successful collaboration.
We are very pleased to welcome Bennet Karetta to the INSPIRE group. He joins the group as a M.Sc. Candidate joint with the TWIST group. We are looking forward to a successful collaboration.
A joint publication by the Organic Spintronics Team showing how key spintronic properties of organic molecules adsorbed at a solid surface may be precisely tuned by modifying the adsorbate structure has been published in Physical Review Letters.
More precisely, experiments performed by our collaborators at Cambridge University (UK), show a broadening of the electron spin resonance (ESR) linewidth upon spin injection from a permalloy surface into thin films of DNTT-based organic molecules. This broadening depends sensitively on the composition and surface bonding of the adsorbate molecules.
With the support of theoretical calculations performed by collaborators at Mons University (BE), significant differences in, e.g., the spin diffusion lengths of the organic adsorbate layers can be inferred from the measured variations in ESR linewidth.
A publication by the Organic Spintronics Team (OST) revising the established method for calculation of molecular spin admixture parameters from first-principles electronic structure theory has been published in Physical Review B. Spin states in a semi-conductor or molecule are a mixture of up and down, because of spin-orbit coupling (SOC). Spin admixture is one of the main ways in which SOC influences the spin dynamics in a molecular material.
The revised method for calculating spin admixture improves on a number of approximations made in the previous method, resulting in greater accuracy and transferability. Still, this method relies on efficient, standard electronic structure theory only, making it easy to implement, and suitable for large-scale calculations.
A publication by the Organic Spintronics Team (OST) revising the established method for calculation of molecular spin admixture parameters from first-principles electronic structure theory has been accepted for publication in Physical Review B. Spin states in a semi-conductor or molecule are a mixture of up and down, because of spin-orbit coupling (SOC). Spin admixture is one of the main ways in which SOC influences the spin dynamics in a molecular material.
The revised method for calculating spin admixture improves on a number of approximations made in the previous method, resulting in greater accuracy and transferability. Still, this method relies on efficient, standard electronic structure theory only, making it easy to implement, and suitable for large-scale calculations.
Sinova and collaborators have published a large review of spin-orbit torques in ferromagnetic and antiferromagnetic systems in Review of Modern Physics. Link here.
A publication by the Organic Spintronics Team (OST) has been published in the Journal of Physical Chemistry C.
This paper presents an application of the recently developed technique for predictions of spin-admixture in molecules. As a computationally robust and efficient, "high-throughput" technique, it is used to describe general trends of in the spin admixture of several classes of molecules, from complex single-molecule magnets to organic polymers. The results emphasize the often counterintuitive variations of molecular spin-orbit coupling with molecular chemical composition and structure.
This paper presents an investigation of ultrafast dynamics in antiferromagnets which is a part of a developing field of an Antiferromagnetic spintronics.By performing magneto-optical pump-probe experiments we excite coherent longitudinal oscillations of the antiferromagnetic order parameter that cannot be described by a thermodynamic Landau-Lifshitz approach. We interpret these oscillations as manifestation of an entanglement of pairs of magnons generated by femtosecond optical pulses. The results open a way to creation and manipulation of quantum entanglement in antiferromagnetic systems at macroscopic scales.